Look at other peoples templates for a starting point. Also, first try overclocking just the CPU or RAM. Once you know that one is stable, go for the other.
You should always have a backup image of your system drive before you overclock. Windows can get corrupted while finding a stable overclock, so it's not necessarily a hardware problem that you can't boot anymore. Did you try with optimized defaults? Also, be sure to check your SATA options and see if it's IDE/ACHI/RAID as it was before.
Looks great.
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