If that is not an E0 stepping, good luck going higher on that voltage, most top out at around 4GHz @ ~1.42v (real load). You can just try various GTL Refs, start with 0.63x on each one and move up to ~ 0.70x on each one. Whichever gives the longest time in orthos without an error is the best setting. However if you can only pass 15mins without an error, I doubt you can get 100% stable with GTL tweaking. id say your cpu is at its limit.
However you could try increasing the vNB, 1.32 is pretty low for DDR3 and that FSB with a quad. Those boards aren't really built for it so you may need to push it. Try 1.40 vNB.
I also assume you have tested the cpu & ram/NB separately using small FFT, large FFT, bootable memtest & windows memtest? What do you pass/fail? Prime is not the only test you need to run, and even with prime you need to run small & large FFT's. Try to give us as much info as possible or else its very hard to know what to suggest to you ok.
Try pulling out 2 ram modules and see if that makes a difference. if it does its your NB at fault.
Have you tested the ram/NB with bootable memtest & windows memtest?
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