Some comments:
The PSU is underspecified for the TEC. You need 30A at 24V, minimum, to run that.
The fan/rad setup is way too weak - holst has covered this above.
You won't be able to power a GPU tec off that PSU as it isn't even powerful enough for the CPU TEC.
Incidentally it's ~720W for the TEC, plus CPU going into the loop, so maybe 850-900W to be cooled. You're not going to make that quiet.
I'd suggest the meanwell SCN-800-24 to power that TEC: http://www.computronics.com.au/meanwell/scn-800/
You still won't be able to power a GPU TEC with it though.
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